Energy and Climate
Energy and ClimateRenewable SystemsEnergy EfficiencySolid-State Lighting Science EFRCOur SSLS EFRC’s Scientific Research Challenges and PublicationsResearch Challenge 6: Beyond Spontaneous Emission

Research Challenge 6: Beyond Spontaneous Emission

This research challenge explores radiative processes that go beyond incoherent emission. For example, although LEDs (based on spontaneously emitted incoherent light) are presently thought of as the source of choice for white light generation. However, coherent light sources have many potential benefits, including ultra-high efficiency, narrow linewidths, improved directionality of light, and the potential to circumvent a phenomenon called efficiency droop. If these benefits could be realized across the visible spectrum, they could provide new routes to overcoming the blue-efficiency, RYG-gap, and higher-functionality-light technology challenges. Our current explorations include both “nonclassical” polariton and “classical” laser sources.

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Reflectivity data from a GaN microcavity showing anticrossing behavior and strong coupling.

However, coherent light sources for solid-state lighting (SSL) are in their infancy, and much exploratory work needs to be done to understand both their potential and their limitations. In this research challenge, we are exploring two approaches to high-efficiency coherent light.

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Four-color laser-based white light source for human-factors study.

The first approach, comprising most of our effort, is focused on polariton sources, which entail coherent light emitted by the polaritons formed from strongly coupled excitons and cavity photons. In the strong-coupling regime, spontaneous emission is replaced by a coherent exchange of energy between excitons and photons, which can lead to polariton lasing. One major challenge is to overcome the phonon bottleneck problem, which, if successfully circumvented, would allow one to use the fast picosecond polariton lifetime to dramatically improve optical efficiency. Though such sources have been pursued for many years, we believe they are poised for breakthroughs with the advent of high-quality InGaN materials and their high exciton-binding energies and oscillator strengths.

The second approach, comprising a smaller effort, is in conventional laser sources, that is, coherent light emitted by stimulated emission in the weak coupling regime. Here, we are exploring the ultimate limits of the most basic characteristics of lasers as applied to SSL. For example, what is the color quality associated with narrow linewidth sources? What are the differences between the fundamental factors that limit efficiencies of lasers (multiple-pass devices) and LEDs (single-pass devices)? How might novel architectures (nanowire lasers) mitigate some of these factors?

Research Participants

  • Dr. Arthur Fischer (SNL) – Principal Investigator – coordinates activities of the team; polariton laser and strong coupling experimental design and measurements.
  • Prof. Steve Brueck and Alexander Neumann (Ph.D Student) (UNM) – Design and implementation of laser set-up for human factors study.
  • Dr. Weng Chow (SNL) – Many-body laser theory calculations.
  • Dr. Daniel Koleske (SNL) – MOVPE growth of GaN and InGaN materials.
  • Dr. Willie Luk (SNL) – Optical measurements and polariton cavity designs.
  • Dr. Jeff Tsao (SNL) – Human factors study, industry perspective, and economic analysis.
  • Dr. Jonathan Wierer (SNL) – Nitride device design, fabrication, and testing.

Research Challenge Publications

  • Carmele, A.; Kabuss, Julia; and Chow, Weng W. Highly-detuned Rabi oscillations in a quantum-dot-microcavity system, Phys. Rev. B, (2013).
  • Chow, Weng W. Are non-classical light sources lasers?, IEEE J. Sel. Top. Quantum Electron., (2012).
  • Lingnau, Benjamin; Ludge, Kathy; Chow, Weng W.; and Scholl, Eckehard Failure of the α factor in describing dynamical instabilities and chaos in quantum-dot lasers, Phys. Rev. E, 86, 065201(R) (2012). [10.1103/PhysRevE.86.065201]
  • Lingnau, Benjamin; Ludge, Kathy; Chow, Weng W.; and Scholl, Eckehard INFLUENCING MODULATION PROPERTIES OF QUANTUM-DOT SEMICONDUCTOR LASERS BY CARRIER LIFETIME ENGINEERING, Appl. Phys. Lett., 101, 131107 (2012). [10.1063/1.4754588]
  • Carmele, A.; Kabuss, Julia; Richter, M.; Knorr, A.; and Chow, Weng W. Quantum optics in a semiconductor quantum dot, Journal of Modern Optics, 58, 1951 (2011). [10.1080/09500340.2011.596630]
  • Neumann, Alexander; Wierer, Jonathan J.; Davis, Wendy; Ohno, Yoshi; Brueck, Steve R. J. ; and Tsao, Jeffrey Y. Four-color laser white illuminant demonstrating high color-rendering quality, Optics Express, 19, A982-A990 (2011). [10.1364/OE.19.00A982]
  • Shelton, David J.; Brener, Igal; Ginn, James C.; Sinclair, Michael B.; Peters, David W.; Coffey, Kevin R.; and Boreman, Glenn D. Strong Coupling between Nanoscale Metamaterials and Phonons, Nano Lett.,, 11, 2104-2108 (2011). [10.1021/nl200689z]
  • Kabuss, Julia; Carmele, A.; Richter, M.; Chow, Weng W.; and Knorr, A. Inductive equation of motion approach for a semiconductor QD-QED: coherence induced control of photon statistics, Phys. Stat. Solidi B, 248, 872 (2011). [10.1002/pssb.201000851]
  • Passmore, Brian S.; Adams, David C.; Ribaudo, Troy; Wasserman, Daniel; Lyon, Stephen; Chow, Weng W.; and Shaner, Eric A. Observation of Rabi Splitting from Surface-plasmon Coupled Conduction-state Transitions in Electrically-excited InAs Quantum Dots, Nano Lett., 11, 338 (2011). [10.1021/nl102412h]
  • Carmele, A.; Richter, M.; Chow, Weng W.; and Knorr, A. Antibunching of Thermal Radiation by a Room-Temperature Phonon Bath: A Numerically Solvable Model for a Strongly Interacting Light-Matter-Reservoir System, Phys. Rev. Lett., 104, 156801 (2010). [10.1103/PhysRevLett.104.156801]
  • Xu, Huiwen; Wright, Jeremy B.; Luk, Ting Shan; Figiel, Jeffrey J. ; Cross, Karen C.; Lester, Luke F.; Balakrishnan, Ganesh; Wang, George T.; Brener, Igal; and Li, Qiming Single-mode lasing of GaN nanowire-pairs, Applied Physics Letters, 101, 113106 (2012). [10.1063/1.4751862]
  • Li, Qiming; Wright, Jeremy B.; Chow, Weng W.; Luk, Ting Shan; Brener, Igal; Lester, Luke F.; and Wang, George T. Single-mode GaN nanowire lasers, Optics Express, 20, 17873-17879 (2012). [10.1364/OE.20.017873]
  • Shan, Qifeng; Dai, Qi; Chhajed, Sameer; Cho, Jaehee; and Schubert, E. Fred Analysis of thermal properties of GaInN light-emitting diodes and laser diodes, Journal of Applied Physics, 108, 084504 (2010). [10.1063/1.3493117]

 

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